Your cherry is very nicely done. I think your method of introducing the mold blocks to the spinning cherry might not work. no matter how ridged you think you have the mold blocks there will be movement of the two halves as you squeezy the two halves together. the halves of the mold must be parallel to the rotation of the cherry to minimize mold block movement.
Maybe rotating the cherry by hand is a good idea to try but again I think the mold halves must be parallel to the rotation of the cherry to get a good mold.
Maybe try to index the mold halves with dowel pins then spot each half with a 1/4" ball end mill then start your cherry by hand as you bring the two halves of the mold blocks together.
I'm just "spit-balling" here so take it for what it's worth -- good luck.