I have a .56cal. T/C SB and a Lyman .550" RB mould for it. With a proper patch, i.e., a thinner patch* than you mentioned, I get decent accuracy (from a rest) @ 25 yd. with 70 - 80gr. FFg. A tow wad fore and aft with that true ..550" RB is also accurate or at least is worth trying (I had a limited sample size). Lastly, although many use a .535" RB with a thicker patch and claim "laser like" or "rifle like" accuracy, I haven't found that to be true. I.e., the .550" RB works better in my gun.
*.0111" - .012" 100% cotton patch material (Sew Classics brand at Jo Ann Fabrics)
P.S. T/C bbl. dimensions vary a bit with the SB. While a .550" RB fits my bore, it may be too large for yours.